Topological modification of the electronic structure by Bi-bilayers lying deep inside bulk Bi2Se3

Abstract

We observe the modified surface states of an epitaxial thin film of a homologous series of (Bi-2)(m)(Bi2Se3)(n), as a topological insulator (TI), by angle-resolved photoemission spectroscopy measurements. A thin film with m : n = 1 : 3 (Bi8Se9) has been grown with Bi-2 bilayers embedded every other three quintuple layers (QLs) of Bi2Se3. Despite the reduced dimension of continuous QLs due to the Bi-2 heterolayers, we find that the topological surface states stem from the inverted Bi and Se states and the topologically nontrivial structures are mainly based on the prototype of 3D TI Bi2Se3 without affecting the overall topological order.